Yellowing older leaves and dying upper branches on orange trees may indicate magnesium deficiency—but first rule out spider mites (check leaf undersides for tiny red dots and fine webbing) and watering issues (both over- and under-watering cause yellowing).
Use magnesium sulfate (Epsom salt) at 1 tablespoon per gallon of water or a light sprinkle (⅛-¼ cup) evenly distributed under the canopy, extending 1-2 feet beyond the drip line. Keep 3-4 inches away from the trunk.
If using a handheld hose, wet soil slowly first, then apply salt solution, then water deeply. Multiple light applications over the season are safer than one heavy dose—excess salt damages roots.
Dolomitic lime supplies magnesium and calcium while raising pH (use only if pH is low). Avoid chemist-grade magnesium; stick with agricultural Epsom salt or dolomitic lime.
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