Your 'Limelight' hydrangeas are struggling in their current pots, and the reason is simple: the containers are far too small for these vigorous shrubs.
A hydrangea tree form needs a substantial root system to support its top growth and flower heads. In a small pot, roots quickly become pot-bound, leading to water stress, nutrient deficiency, and the drooping you see after rain. The soil volume simply can't hold enough moisture for the plant's needs.
For a 'Limelight' hydrangea trained as a standard, a minimum of a 24-inch diameter pot is required, but a 30-inch wide container is far better. Even then, annual root pruning and top-dressing with fresh compost will be necessary to maintain vigor. The ideal long-term solution is planting them in the ground where they can thrive with minimal intervention.
With proper space, 'Limelight' will reward you with massive, lime-green to pink flower panicles for years.
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